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Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms.
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The dipole moment function was calculated as described in Ref. Aymar and Dulieu 2005 . The transition dipole moment varies not more than 10 % around an average value of 9.9 Debye over the relevant distances
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This clearly indicates the excitation of a single parity component of B Π 1 {}^{1}\Pi : for even rotational levels in Π 1 {}^{1}\Pi , the odd parity component decays only via the Q-branch into Σ + 1 {}^{1}\Sigma^{+} while the even parity component decays via the P- and R-branch. Odd parity levels of Π 1 {}^{1}\Pi only couple to even partial waves of the scattering continuum. As J ′ J^{\prime} =2 can not be excited from continuum states with angular momentum ℓ \ell =0 via a dipole transition, the excitation can only originate in ℓ \ell =2, which suggests the presence of a d d -wave shape resonance. Note that the Λ \Lambda doubling of the PA levels is on the order of 1MHz Stein et al. 2008
Cited in the paper.
The strong d d -wave contribution to the PA via B Π 1 {}^{1}\Pi , v ′ v^{\prime} =4, J ′ J^{\prime} =2 couples also to the negative parity component of B Π 1 {}^{1}\Pi , v ′ v^{\prime} =4, J ′ J^{\prime} =1. Decay from this component populates X Σ 1 {}^{1}\Sigma , v ′′ v^{\prime\prime} =0, J ′′ J^{\prime\prime} =0,2 as observed. The additional population of J ′′ J^{\prime\prime} =1 can be explained by p-wave contributions to the continuum wave function
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